Instytut Podstawowych Problemów Techniki
Polskiej Akademii Nauk

Partnerzy

Qin Lin


Ostatnie publikacje
1.  Nwaji N., Akinoglu E.M., Lin Q., Teshome Tufa L., Sharan A., Singh N., Wang X., Giersig M., Lee J., Surface Modulation of Fe3O4 Confined in Porous Molybdenum-Based Nanoplatform for Enhanced Hydrogen Production, Energy Technology, ISSN: 2194-4296, DOI: 10.1002/ente.202201061, Vol.11, No.2, pp.2201061-1-9, 2023

Streszczenie:
The integration of different precursor components to form single nanostructures via one-step synthesis process is mostly restricted by the compatibility and complexity of components. Herein, a highly uniform, spherical, hollowed, and hierarchical iron oxide-wrapped Mo–polydopamine is synthesized using a one-pot liquid-phase reaction at room temperature. Mo2C is doped with Fe3O4 to harness the rich electrons in Fe dopants for effective lowering of the unoccupied d-orbitals in Mo. The surface conductivity of the as-prepared nanostructures is enhanced by decorating them with gold nanoparticles utilizing strong interaction of Au and amine. The nanocomposites are converted into carbidic hollowed structures via an annealing process without any distortion in morphology. The well-organized structure and nanosize of the particles provide efficient catalytic performance for hydrogen evolution reaction in acidic media. MoFe–C@Au exhibits a very positive onset potential of 2 mV, low Tafel slope of 50.1 mV dec^-1, and remarkable long- term stability.

Słowa kluczowe:
electrocatalysts,hierarchical syntheses,hydrogen evolution,molybdenum,polydopamine

Afiliacje autorów:
Nwaji N. - inna afiliacja
Akinoglu E.M. - University of Melbourne (AU)
Lin Q. - inna afiliacja
Teshome Tufa L. - inna afiliacja
Sharan A. - inna afiliacja
Singh N. - inna afiliacja
Wang X. - inna afiliacja
Giersig M. - IPPT PAN
Lee J. - Lexington High School (US)
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